通过使用多个溶解气体的高分辨率时间序列来量化地下水-流-大气层连续的碳循环
Chuan Wang1,2,3, Matthias S Brennwald3, Yueqing Xie1,2
1Key Laboratory of Surficial Geochemistry, Ministry of Education, School of Earth Sciences and Engineering, Nanjing University, Nanjing 210023, China.
Environmental science & technology
|August 29, 2023
概括
地下水对碳排放产生重大影响,提供二氧化碳和甲. 高分辨率的溶解气体分析揭示了在地下水-流-大气连续体 (GSAC) 中的动态碳循环.
科学领域:
- 环境科学 环境科学
- 地质化学 地质化学
- 生物地质化学生物地质化学
背景情况:
- 在地下水-流-大气连续体 (GSAC) 中量化碳循环对于全球碳预算至关重要.
- 在GSAC中,结合的碳交换和转移带来了重大的量化挑战.
研究的目的:
- 在一个代表性的GSAC截面中解开碳循环过程.
- 用高时空分辨率量化碳交换和转移.
主要方法:
- 获得溶解气体 (He, Ar, Kr, O2, CO2, CH4) 的高分辨率时间序列.
- 使用数值模拟来分析气体度和碳动态.
- 研究了流体代谢和碳酸盐沉/溶解的日间变化.
主要成果:
- 地下水约占二氧化碳流的60%和CH4输入流的30%.
- 大气中的二氧化碳和四氧化碳排放被这些地下水输入所支持.
- 河流代谢的日间变化推动了显著的碳酸盐沉和溶解周期.
结论:
- 溶解的气体作为有效的标志物用于辨别和量化GSAC碳循环.
- 高分辨率的时间序列对于理解生物地化学过程的日间变异性至关重要.
- 这项研究提供了对整个GSAC的碳循环的机制性理解.
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