在不同大气层中重复脉冲气液排放:从排放特征到等离子体-液体相互作用
1College of Electrical Engineering and Control Science, Nanjing Tech University, Nanjing, Jiangsu, 211816, China. wang_sen@njtech.edu.cn.
Physical chemistry chemical physics : PCCP
|September 15, 2023
概括
在等离子体液体排放中的气通过到达液体,显著提高了相互作用效率. 不同的气体,如和,表现出不同的等离子体特性和化学生产,影响应用.
科学领域:
- 等离子体科学与工程等离子体科学与工程
- 化学物理 化学物理
- 表面科学是一门学科.
背景情况:
- 气液排放对于各种应用中的等离子体液相互作用至关重要.
- 工作气体的选择显著影响排放特性和效率.
- 了解气体特异性等离子体特性对于优化这些系统至关重要.
研究的目的:
- 为了研究不同工作气体 (,,) 对脉冲针到水气液排放的影响.
- 探索放电模式,进化过程和等离子体特性.
- 阐明工作气体在化学物种生成中的作用.
主要方法:
- 利用电压电流波形和强化电荷合装置 (ICCD) 成像来分析放电行为.
- 使用光学发射光谱 (OES) 来描述等离子体的特性.
- 进行与二甲基硫氧化物和没有二甲基硫氧化物的实验,以研究化学生产途径.
主要成果:
- 阿贡排放扩展到液体中,与和不同,增强了血与液体的相互作用.
- 包括激发物种在内的等离子体特性受到水蒸气和工作气体的强烈影响.
- 阿贡和排放与二甲基硫氧化物产生NO2-和NO3-,而主要产生NO3-.
结论:
- 在这种放电配置中,是最大限度地提高等离子体-液体相互作用效率的优势.
- 工作气体的选择对等离子体化学和OH,NO,NO2-和NO3-等反应性物种的产生产生重大影响.
- 这项研究为为特定应用量身定制气液排放提供了基础的见解.
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