化佩洛夫斯基特中持久和准持久的旋转纹理是由单轴应力诱导的
Ravi Kashikar1, Abduljelili Popoola1, Sergey Lisenkov1
1Department of Physics, University of South Florida, Tampa, Florida 33620, United States.
The journal of physical chemistry letters
|September 19, 2023
概括
研究人员发现,对混合有机-无机矿施加单轴应力可以创建持久的旋转纹理,这对旋转电子学至关重要. 这一发现为开发柔性和性自旋电子设备打开了大门.
科学领域:
- 材料科学 材料科学 材料科学
- 凝聚物质物理学 凝聚物质物理学
- 固态化学 固态化学
背景情况:
- 持久的旋转纹理对于旋转电子是必不可少的,使运载机的旋转寿命长.
- 由于需要精确的旋转动量合参数,实现这些纹理是具有挑战性的.
研究的目的:
- 通过单轴应力在混合有机-无机矿中诱导持久自旋纹理的潜力.
- 为了探索在机械应力下在MPSnBr3中旋转纹理的调性.
主要方法:
- 用密度函数理论 (DFT) 模拟来建模材料的电子和自旋特性.
- 这项研究的重点是甲基酸 (CH3PH3) SnBr3 (MPSnBr3) 材料.
主要成果:
- MPSnBr3在导电带最小附近呈现持久旋转纹理,在价值带最大附近呈现Rashba类型纹理.
- 单轴应力 (拉力或压力) 改变了价值带旋转纹理,导致准持久或纯Rashba类型.
- 该材料表现出灵活性,类似的反应和显著的压电特性.
结论:
- 单轴应力提供了一种可行的方法,可以在MPSnBr3.3中设计持久自旋纹理.
- 可调节的旋转纹理和机械灵活性的独特组合表明了新的灵活的旋转电子应用的潜力.
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