在倾斜的表面上升级气液吸收中的分散
Morteza Dejam1, Hassan Hassanzadeh2
1Department of Energy and Petroleum Engineering, College of Engineering and Physical Sciences, University of Wyoming, 1000 E. University Avenue, Laramie, Wyoming 82071-2000, USA.
Physical review. E
|October 18, 2023
概括
这项研究模拟了倾斜液体薄膜中的气体吸收,揭示了三个质量转移区域. 一个最佳的液体流速 (Peclet数) 最大化了气体吸收效率.
科学领域:
- 化学工程是化学工程的重要组成部分.
- 流体动力学 流体动力学
- 质量转移是指质量转移.
背景情况:
- 液中的气体吸收对于工业分离过程至关重要.
- 了解质量转移动力学对于过程优化至关重要.
- 泰勒-阿里斯分散理论为分析运输现象提供了一个框架.
研究的目的:
- 为在倾斜表面的粘性液体薄膜中开发气体吸收的升级模型.
- 分析向,分散和反应动力学对质量转移的影响.
- 为了确定最大限度地提高气体吸收的最佳运行条件.
主要方法:
- 泰勒-阿里斯分散理论的扩展.
- 开发一个减少顺序的向导-分散-反应模型.
- 雷诺兹分解和横截面平均值的应用.
- 升级模型的分析解决方案.
主要成果:
- 确定三个质量转移区域:向导主导,过渡和吸收主导.
- 在吸收主导区域中确定缩放关系Sh∼Da^{1/2}.
- 在前两个区域观察钟形 (高斯式) 谢伍德数对佩克莱数的依赖性,表明质量转移的最佳佩克莱数.
结论:
- 升级模型准确地预测了气体吸收动力学和质量转移.
- 存在一个最佳的佩克莱特数,可以在特定的流程中最大限度地实现气液质量转移.
- 这些发现适用于工业分离过程,涉及倾斜表面上的气液相互作用.
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