电子运输二分化在生物阳极中与代谢转移到酸盐还原
Yinchi Xu1, Lanhua Liu1, Erhuan Sun1
1School of Ecology & Environment, Zhengzhou University, Zhengzhou, Henan 450001, China.
The Science of the total environment
|October 26, 2023
概括
微生物电化学技术将电子流从电极转移到酸盐,降低了效率. 这种代谢转移降低了电子转移,并增加了由于外电原体损失的生物膜阻力.
科学领域:
- 微生物的电化学
- 生物电化学系统 生物电化学系统
- 环境微生物学环境微生物学
背景情况:
- 微生物电化学技术 (MET) 中的生物阳极性能对于能量回收至关重要.
- 电子运输分支,电子被指向不同的受体,影响MET效率.
- 了解代谢转变是优化生物阳极功能的关键.
研究的目的:
- 为了研究从当前生产到脱的代谢转变期间的生物阳极反应.
- 分析电子转移效率,微生物群落和结构的变化.
- 为了阐明电子转移二叉反应对替代电子受体的机制.
主要方法:
- 循环电压测量和电化学阻抗光谱学被用来评估电子传输路径.
- 使用共聚焦成像来分析微生物结构和细胞活力.
- 在代谢转移之前和之后对生物模块性能进行比较分析.
主要成果:
- 在脱化过程中,用于减电极的电子转移效率下降了大约17%.
- 生物膜阻力和电荷转移阻力显著增加.
- 混焦成像显示出高比例的非活性细胞,表明外电原体的损失.
结论:
- 从电极还原到酸盐还原的代谢转移导致了电子运输的分叉.
- 观察到的性能下降主要归因于外电致细菌的丧失.
- 这项研究提出了在生物阳极中电子转移分支的机制.
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