通过界面电荷转移对分层反铁磁体的工程磁相
Kaichen Xie1, Xiao-Wei Zhang1, Di Xiao1,2
1Department of Materials Science and Engineering, University of Washington, Seattle, Washington 98195, United States.
ACS nano
|November 14, 2023
概括
范德瓦尔斯异构结构中的界面电荷转移可以切换磁相. 在石墨烯上堆叠抗铁磁CrSBr会诱导铁磁相,从而使自旋电子的门控制磁性成为可能.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 量子化学 是一个量子化学.
背景情况:
- 由于接口合,范德瓦尔斯的异构结构表现出独特的特性.
- 二维磁铁为先进的自旋电子设备提供了潜力.
研究的目的:
- 通过界面电荷传输来研究2D磁铁中的磁相操纵.
- 探索异构结构中从反铁磁到铁磁相的过渡.
主要方法:
- 第一个原则计算模型 CrSBr / 石墨烯异构结构.
- 连接单层的有效模型,以分析磁相转换.
主要成果:
- 在石墨烯上堆叠反铁磁双层 CrSBr 诱导过渡到铁磁阶段.
- 接口电荷转移增强铁磁,由电子或孔载体驱动.
- 过渡过程涉及一个旋转转向的过程,允许门控制的非线性磁力.
结论:
- 接口电荷转移是范德瓦尔斯异构结构中调整磁相的强大机制.
- 这项工作为设计新型自旋电子应用程序开辟了道路.
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