使用稳定的Si同位素探测地球表面的反应性二氧化循环:质量平衡,流动和深度时间影响
Shaily Rahman1,2, Elizabeth J Trower1
1Department of Geological Sciences, University of Colorado Boulder, Boulder, CO, USA.
Science advances
|December 6, 2023
概括
这项研究证实了现代的二氧化循环是在同位素质量平衡中. 地质水库中的 (Si) 同位素值准确地反映了古气候和古生产力,验证了它们作为代理的使用.
科学领域:
- 地质化学 地质化学
- 古气候学 古气候学
- 生物地质化学生物地质化学
背景情况:
- 地质水库中的 (Si) 同位素值 (δ30Si) 被用作古气候和古生产力的代理值.
- 应用程序假设地表地球Si同位素预算与大量酸盐地球的质量平衡.
- 这意味着时间 δ30Si 趋势反映了库流量的变化.
研究的目的:
- 为了测试表面地球Si同位素预算中的质量平衡假设.
- 为了评估不同库的 δ30Si 值之间的关系.
- 在现代的循环中调和Si流和同位素特征.
主要方法:
- 从现代的二氧化来源和沉积点收集的 δ30Si 数据的汇编.
- 应用一个反向模型来评估质量平衡.
- 分析酸盐矿物质的气候变化和陆地二氧化储存.
主要成果:
- 反向气候变化产品的 δ30Si 值必须与藻的值相匹配,从而挑战了先前的假设.
- 每年大约1018特拉莫尔的气候变化释放的Si储存在陆地水槽中.
- 现代的二氧化循环被证明是在同位素质量平衡中.
结论:
- 这项研究验证了地质 δ30Si 作为古气候和古生产力代理物的使用.
- 它完善了对气候变化,逆气候变化和生物水槽之间的Si同位素分区的理解.
- 这些发现证实了当代二氧化循环的同位素质量平衡.
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