在Fe (III) 和硫酸盐降低条件下,本土微生物在本托尼特中的温度依赖微生物反应
Su-Young Park1, Yidan Zhang1, Edward J O'Loughlin2
1Department of Earth and Environmental Sciences, Korea University, Seoul 02841, South Korea.
Journal of hazardous materials
|December 28, 2023
概括
作为废核燃料储存材料的本托尼特中的微生物活动受温度的影响. 较高的温度 (50°C) 有利于硫酸盐的减少,而较低的温度 (18°C) 有利于铁的减少和特定的发酵途径.
科学领域:
- 地质微生物学的生物.
- 环境科学 环境科学
- 核废物管理 核废物管理
背景情况:
- 石是废核燃料 (SNF) 储存库中工程屏障的关键材料.
- 储存库的密封创造了无氧条件,可能刺激微生物活动.
- 放射性核酸的衰变产生热量,这可能会影响本托尼特内的微生物过程.
研究的目的:
- 为了研究温度对本托尼特微生物活动的影响.
- 了解温度如何影响微生物发酵和无氧呼吸在仓库环境中.
主要方法:
- 使用WRK顿石,乳酸盐 (电子捐赠物) 和硫酸盐和/或铁 (Fe(III)) (电子接受物) 制备了微观宇宙.
- 在两个温度下进行化:18°C和50°C.
- 监测了微生物的新陈代谢和减少过程.
主要成果:
- 当地的微生物在18°C和50°C时都能降低硫酸盐和Fe (III),但速度和程度不同.
- 乳酸盐在两种温度下发酵为酸盐;酸盐也在18°C时产生.
- 在18°C时Fe (III) 的降解更高,而在50°C时硫酸盐的降解更高.
结论:
- 温度显著影响微生物的代谢途径和顿石中的电子受体利用.
- 热友和/或代谢灵活的微生物在本托尼特的生态化学循环中发挥作用.
- 存储库的设计必须考虑到温度依赖的微生物活动,以确保SNF存储库的长期稳定性.
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