在ANAMMOX颗粒污泥中Ca2+粘附导致的较大的氧酸聚合是由高溶解氧气引起的
Mu Yuan1, Qiu Shan2, Mengqi Fu1
1School of Environment, Harbin Institute of Technology, Harbin, 150090, China.
Chemosphere
|January 10, 2024
概括
溶解氧的波动改变无氧氨氧化 (ANAMMOX) 污泥,导致离子粘附,形成酸. 这影响了污泥形态和微生物群落,为防止污泥在废水处理中的恶化提供了一种策略.
科学领域:
- 环境科学 环境科学
- 微生物学 微生物学
- 生物技术是生物技术.
背景情况:
- 无氧氨氧化 (ANAMMOX) 是一个关键的可持续过程,用于从城市废水中去除 (NH4+-N).
- 泥形态对于有效的ANAMMOX性能至关重要,但影响其稳定性的因素需要进一步调查.
研究的目的:
- 为了研究溶解氧 (DO) 波动对anammox颗粒污泥形态和组成的影响.
- 在不同的DO条件下识别污泥恶化背后的机制.
- 探索在ANAMMOX工艺中保持污泥稳定性的策略.
主要方法:
- 使用扫描电子显微镜 (SEM),数码相机成像,能量分散光谱仪 (EDS) 和X射线衍射 (XRD) 来描述污泥形态.
- 对细胞外聚合物物质 (EPS) 的分析,特别是蛋白质与多糖的比率 (PN/PS).
- 微生物群体分析以确定在不同DO暴露下的主导属.
主要成果:
- 交替溶解氧 (DO) 水平诱导离子 (Ca2+) 粘附于污泥表面,形成酸并改变污泥形态.
- 氧酸盐覆盖了原始污泥的孔隙,影响了其结构.
- 在氧气暴露下观察到PN/PS比率的下降,微生物群落发生了转移,norank_f_A4b和Nitrolancea在不同的时间点占主导地位.
结论:
- 由于离子粘附和氧酸盐的形成,DO的变化显著影响了anammox颗粒污泥的形态.
- 观察到的EPS和微生物群落的变化凸显了ANAMMOX对氧气水平的敏感性.
- 操纵DO和Ca2+度是一个可行的策略,以防止城市废水ANAMMOX系统中的污泥恶化.
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