的生物地化学循环与微生物功能和有机物分子组成的盆地规模动态有关
Xianjun Xie1, Lu Yan1, Shige Sun2
1State Environmental Protection Key Laboratory of Source Apportionment and Control of Aquatic Pollution, Ministry of Ecology and Environment, Wuhan 430074, China; MOE Key Laboratory of Groundwater Quality and Health, China University of Geosciences, Wuhan 430078, China.
Water research
|January 14, 2024
概括
地质性 (As) 在地下水中的污染是一个全球性的健康问题. 微生物活动和溶解有机物影响AS释放和固定在不同的氧化还原条件下,影响其区域分布.
科学领域:
- 环境科学 环境科学
- 地质化学 地质化学
- 微生物学 微生物学
背景情况:
- 地质性 (As) 污染的地下水对全球健康构成重大风险.
- 了解控制地下水中氧气循环的复杂生态化学过程至关重要.
- 之前的研究缺乏对微生物相互作用和As生物地质化学的区域划分的全面了解.
研究的目的:
- 阐明地质微生物相互作用网络控制高As地下水中的生物地质化学途径.
- 研究氧化还原条件和溶解有机物对动员和不动化的影响.
- 建立在地下水中循环的理论模型.
主要方法:
- 集成的现场水地化学监测.
- 超基因组分析以确定微生物功能基因.
- 超高分辨率质谱仪 (FT-ICR MS) 用于溶解有机物质的表征.
主要成果:
- 在氧化到弱降解环境中,酸盐降解和硫酸盐降解基因抑制了含有的铁矿物质溶解,降低了水平.
- 在微弱到中度减少的环境中,硫酸盐减少和铁运输基因促进了铁矿物质的溶解和释.
- 在强烈减少的条件下,甲循环基因增强了As调动,部分是通过气态甲基的形成.
结论:
- 在地下水中的迁移和固定是由盆地规模的微生物功能和溶解有机物成分控制的.
- ,硫,铁和碳的氧化还原循环显著影响的生物地球化学.
- 这项研究为循环的生物地球化学网络提供了新的见解,并为其理解提供了一个理论模型.
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