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Updated: Jul 4, 2025

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切换电催化进化途径通过铜氨酸的电子调

Xinyang Peng1, Mengchun Zhang1, Haonan Qin1

  • 1Key Laboratory of Applied Surface and Colloid Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shaanxi Normal University, Xi'an, 710119, China.

Angewandte Chemie (International ed. in English)
|February 5, 2024
PubMed
概括

铜氨酸的电子调节可以控制进化反应 (HER) 路径. 这项研究表明,通过受控合成,可以将催化活性物种从Cu(I) 转换为Cu(0).

关键词:
铜氨酸是铜氨酸的一种.电子调电子调的进化 的进化分子电催化学分子电催化学反应机制的反应机制

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The absorption of UV–visible light by conjugated systems causes the promotion of an electron from the ground state to the excited state. Consequently, photochemical electrocyclic reactions proceed via the excited-state HOMO rather than the ground-state HOMO. Since the ground- and excited-state HOMOs have different symmetries, the stereochemical outcome of electrocyclic reactions depends on the mode of activation; i.e., thermal or photochemical.
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