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可扩展的干燥工艺,用于制造Na超电子导体类型的固体电解质板.

Suyeon Kim1,2, Seongmin Shin1,2, Dae Soo Jung1

  • 1Energy & Environmental Division, Korea Institute of Ceramic Engineering & Technology (KICET), 101 Soho-ro, Jinju-si, Gyeongsangnam-do 52581, Republic of Korea.

ACS applied materials & interfaces
|February 21, 2024
PubMed
概括
此摘要是机器生成的。

本研究介绍了一种无溶剂干燥工艺,用于为全固态电池制造高密度,灵活的超离子导体固体电解质板. 使用3%重量的聚四乙烯 (PTFE) 粘合剂进行优化,该材料实现了1.03mS cm-1的高离子导电性.

关键词:
这里是纳西康尼.干燥制造工艺 干燥制造工艺灵活的纸板是灵活的纸板.高离子导电性的高离子导电性.固体电解质是一种固体电解质.

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科学领域:

  • 材料科学 材料科学 材料科学
  • 电化学 电化学 电化学
  • 固态化学 固态化学

背景情况:

  • 全固态电池的商业化取决于成本效益高的大量生产固体电解质.
  • 目前用于氧化物固体电解质的方法通常涉及溶剂,并限制活性物质的度.

研究的目的:

  • 开发一种环保,无溶剂的干燥工艺,用于制造高密度,灵活的基于氧化物的超离子导体固体电解质板.
  • 研究粘合剂含量和颗粒大小对通过干燥工艺生产的固体电解质板的性能的影响.

主要方法:

  • 使用新型干燥工艺制造固体电解质板,避免使用溶剂.
  • 使用聚四乙烯 (PTFE) 作为粘合剂,通过剪切力转化为线状结构以提高灵活性.
  • 优化干燥工艺,使绿色纸张中的固体电解质粉末含量增加到95%以上.
  • 研究粘合剂含量 (特别是3重%的PTFE) 和细磨固体电解质粉对离子导电性的影响.

主要成果:

  • 干燥工艺使得与传统的湿工艺相比,绿色板材的密度明显更高.
  • 干燥工艺允许固体电解质粉末含量超过95%的重量,而潮湿工艺的重量限制为50%.
  • 优化的固体电解质板 (3重量%的PTFE粘合剂,精细磨粉) 呈现出最高的总离子导电率,达到1.03mS cm-1.

结论:

  • 无溶剂干燥工艺对于生产高密度,灵活的基于氧化物的固体电解质板来说是有效的.
  • 这种方法显著增加了固体电解质含量,并提高了密度,这对电池性能至关重要.
  • 这种优化的材料在全固态电池中的应用中显示出有前途的离子导电性.