π 卡戈梅超导体中的相间层转移和堆叠故障 CsV_{3}Sb_{5}
Feng Jin1, Wei Ren2, Mingshu Tan2
1Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190, China.
Physical review letters
|February 23, 2024
概括
卡戈梅超导体CsV_{3}Sb_{5}中的层叠对其性能产生影响. 拉曼测量显示了一个2c分级的顺序阶段和一个堆叠的顺序-失序过渡,影响超导.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 超导电性 超导电性 超导电性
背景情况:
- 分层材料的性能可以通过堆叠来调整.
- CsV_{3}Sb_{5}是一个kagome超导体,呈现3D电荷密度波 (CDW) 阶段.
- 在CsV_{3}Sb_{5}CDW阶段的外平面调制仍然不清楚.
研究的目的:
- 在CsV_{3}Sb_{5}中研究CDW相的外平面调制.
- 确定结构过渡及其与堆叠的关系.
- 了解超导和CDW顺序之间的相互作用.
主要方法:
- 偏振依赖的拉曼光谱学.
- 温度依赖的拉曼光谱法.
- 分析音声模式和热歇斯底里.
主要成果:
- 观察到C_{6}旋转对称性的破坏,表明有三个不同的域.
- 确认了一个2c分级顺序相,在相邻层之间有一个π相位移.
- 确定了在65K处的第一阶层结构阶段过渡,归因于堆叠秩序-混乱.
- 通过Cs相关的声模式歇斯底里存在堆叠故障的证据.
结论:
- 堆叠自由度对于 CsV_{3}Sb_{5} 属性至关重要.
- CDW阶段的特点是平面外的摇摆.
- 一个堆叠的顺序-混乱过渡影响材料的行为.
- 这些发现提供了对超导-CDW纠的结构性见解.
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