旋转和轨道角动量的超快形前行,由初级铁磁磁体中的循环极化激光脉冲诱导
Junjie He1, Thomas Frauenheim2, Shuo Li3
1Department of Physical and Macromolecular Chemistry, Faculty of Science, Charles University, Prague 12843, Czech Republic.
The journal of physical chemistry letters
|February 26, 2024
概括
这项研究表明,在激光诱导的去磁化中,轨道角动量 (OAM) 显著大于旋转角动量 (SAM). 在Fe,Co和Ni中观察到OAM和SAM的奇拉性和超快的先行动态.
科学领域:
- * 凝聚物质物理学 凝聚物质物理学
- * 超快磁力 超快磁力 超快磁力
- * 计算材料科学 计算机材料科学
背景情况:
- * 旋转 (SAM) 和轨道 (OAM) 角动量动力学在去磁化中至关重要.
- * 从历史上看,重点是总角动量,对组件动态的关注较少.
研究的目的:
- * 调查SAM和OAM的诱导x和y组件.
- *分析循环极化激光脉冲对这些动态的影响.
- * 为了比较SAM和OAM precession与demagnetization的幅度和时间尺度.
主要方法:
- *实时的时间依赖密度函数理论 (rt-TDDFT) 模拟.
- *对受极化激光脉冲的铁磁材料 (Fe,Co,Ni) 进行建模.
主要成果:
- *OAM大小是大小大于SAM的一个数量级,表示主导轨道响应.
- * 循环左 (σ+) 和右 (σ-) 极化脉冲诱导SAM和OAM的明显的性前行模式.
- *OAM和SAM的先行发生在超快的时间尺度上,先于去磁化和光学诱导旋转转移 (OISTR) 效应.
结论:
- * 轨道角运动量在超快激光诱导的去磁化中起着主导作用.
- * 角动量动态中的奇拉性与激光极化直接相关.
- *SAM和OAM的超快速前行提供了对磁性材料中激光物质相互作用的新见解.
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