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关于基于半碳化的单原子催化剂的第一原则见解:单原子迁移和减少氧气的机制

Xiangyu Zhu1, Mingqi He2, Xing Chen1

  • 1Institutes of Physical Science and Information Technology, Anhui University, Hefei, Anhui 230601, China.

The journal of physical chemistry letters
|March 5, 2024
PubMed
概括

Tungsten 半碳化物支持的单原子催化剂表现出动态的单原子迁移,揭示出一种新的活性相进化途径. 这种自我优化增强了氧降解反应的催化活性和稳定性.

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Alkenes are converted to 1,2-diols or glycols through a process called dihydroxylation. It involves the addition of two hydroxyl groups across the double bond with two different stereochemical approaches, namely anti and syn. Dihydroxylation using osmium tetroxide progresses with syn stereochemistry.
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