多相反应流和质量转移在功能化微流体多孔介质中的可视化
Hangkai Wei1,2, Xin Sha1, Li Chen1
1Key Laboratory of Thermo-Fluid Science and Engineering of MOE, School of Energy and Power Engineering, Xi'an Jiaotong University, Xi'an, Shaanxi, 710049, China.
Small (Weinheim an der Bergstrasse, Germany)
|March 13, 2024
概括
这项研究可视化了工程孔隙介质中的多相反应流. 水力动力学不稳定性会产生偏好的流动路径,影响反应速率和泡形成,特别是在异质结构中.
科学领域:
- 地质化学 地质化学
- 化学工程是化学工程的重要组成部分.
- 流体动力学 流体动力学
背景情况:
- 多相反应流在多孔介质中对于自然和工业过程至关重要.
- 了解这些复杂的相互作用是优化各种应用程序的关键.
研究的目的:
- 在制造的多元组件矿物质多孔介质中研究多相反应流.
- 量化不同条件对流动动态和反应路径的影响.
主要方法:
- 矿物质多孔介质的制造,使用微通道中的光刻法.
- 微流体学实验以捕捉实时的反应流.
- 甲基紫色2B用于可视化酸度场.
- 先进的图像处理用于定量阶段分布分析.
主要成果:
- 低酸度导致单相反应.
- 较高的酸度会导致多相水力学不稳定性,形成偏好的流道.
- 增加输入速度加速反应,但减少了泡的产生.
- 较低的入口速度会产生更多的气泡,阻碍流动和反应.
- 不同质的结构 (骨折,腔) 重定向流动并促进优选路径.
结论:
- 工程孔隙介质使得多相反应流的详细研究成为可能.
- 水力动力学不稳定性是优先流和反应的关键驱动因素.
- 流速和多孔结构显著影响反应动态和气泡行为.
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