大气中异烯测量显示,南大洋的排放量大于预期
Valerio Ferracci1,2, James Weber3,4, Conor G Bolas5,6
1Cranfield Environment Centre, Cranfield University, College Road, Cranfield, UK. v.ferracci@cranfield.ac.uk.
Nature communications
|March 23, 2024
概括
南洋海洋异烯排放量被模型低估了. 新的测量显示,边缘冰区的高度异烯,影响大气化学和气候.
科学领域:
- 大气化学 大气化学
- 海洋-大气层相互作用
- 气候科学 气候科学
背景情况:
- 异烯是一种有反应性的大气微量气体,由陆地和海洋生物排放.
- 由于有限的长期测量,人们对海洋异烯流的了解很差.
- 异烯影响大气组成,包括臭氧,甲和气溶的形成.
研究的目的:
- 在夏季在南大洋分析大气中异烯度.
- 在高度海洋环境中识别显著的异烯来源.
- 通过使用地球系统模型,评估当前的海对空异烯流量估计.
主要方法:
- 大气中的异烯度在南大洋四个月内被测量.
- 数据分析的重点是确定高度区域和潜在的排放源.
- 用英国地球系统模型将观测结果与模型估计进行比较.
主要成果:
- 在罗斯海和阿蒙森海的边缘冰区观察到最高的异烯度 (>500 ppt).
- 目前的海对空异烯流量估计低估了观察到的度超过20倍.
- 一个白天的异烯源是必要的,以使模型模拟与观测数据相协调.
结论:
- 边缘冰区是一个重要的,以前被低估的高度大气异烯来源.
- 低估的异烯排放影响了气候模型和我们对偏远地区大气氧化的理解.
- 修订的排放清单对于准确建模大气组成及其气候影响至关重要.
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