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单原子催化剂定制陶膜,用于选择性去除新出现的有机污染物

Jiaxuan Yang¹, Jing Zhao¹, Hesong Wang¹

¹State Key Laboratory of Urban Water Resource and Environment, School of Environment, Harbin Institute of Technology, Harbin, 150090, PR China.

Environmental science and ecotechnology

|April 8, 2024

概括

一种新型的单原子催化剂陶膜与氧硫酸盐有效地从废水中去除新出现的有机污染物. 这种先进的氧化过程还防止了膜污染,提高了水的再利用可持续性.

科学领域:

环境科学环境科学
材料科学材料科学材料科学
化学工程是化学工程的重要组成部分.

背景情况:

再利用水对于解决水资源短缺和增加废水至关重要.
超过 (UF) 是一种低能耗的水处理方法,但与新出现的有机污染物 (EOC) 斗争.
环氧化产品对化废水质量和工艺可持续性构成挑战.

研究的目的:

开发一种有效的方法来去除EOC并减轻废水处理中的污染.
提高超过工艺的性能和可持续性,以重复利用水.

主要方法:

制造一个单原子催化剂量身定制的陶膜 (Co1-NCNT-CM).
Co1-NCNT-CM与激活过氧硫酸盐 (PMS) 系统的集成.
研究EOC降解的界面反应机制和催化途径.

主要成果:

Co1-NCNT-CM/PMS系统实现了超过90%的和硫胺的去除.
一个界面反应机制通过排斥自然有机物来缓解膜污染.
在Co-N3-C活性位点单点氧气生成促进了选择性EOC氧化.

结论:

Co1-NCNT-CM/PMS系统在有机污染清除和膜维护方面提供了卓越的性能.
这个综合系统代表了可持续废水处理和水再利用的重大进步.
这些发现为先进的水资源管理框架中有针对性的EOC去除开辟了新的途径.

关键词:

接口响应接口响应多层功能区是多层功能区.过氧单硫酸盐的激活方式选择性氧化是一种选择性氧化.一个原子的催化陶膜.

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