通过量子发射器和金属纳米粒子杂的纳米波导体中光发光的过渡性研究
Grant Brassem1, Mahi R Singh1, Sergey Yastrebov2
1Department of Physics and Astronomy, The University of Western Ontario, London, N6A 3K7, Canada.
概括
我们开发了一种纳米波导光学特性理论,展示了双极-双极相互作用和表面等离子体极子控制短暂的光发光振荡,从而实现了新的纳米开关应用.
科学领域:
- *纳米光子学和量子光学
- * 材料科学与工程 * 材料科学与工程
背景情况:
- * 带有量子发射器的纳米波导和金属纳米粒子表现出复杂的依赖时间的光学特性.
- * 了解瞬态光发光 (PL) 对于开发先进的纳米尺度设备至关重要.
研究的目的:
- * 开发纳米波导体中短暂光发光的理论模型.
- * 调查双极双极相互作用 (DDI) 和表面等离子体极子 (SPPs) 对光学特性的影响.
- * 探索纳米级光学设备的潜在应用.
主要方法:
- *采用密度矩阵方法来建模激子群密度和短暂光发光.
- *金属纳米粒子和表面等离子体极子之间的嵌入式双极-双极相互作用.
- * 验证了理论模型与来自CdSe/ZnS量子点和Ag纳米基纳米混合物的实验过渡PL数据.
主要成果:
- * 该理论准确地预测了实验中的瞬态光发光的数据.
- *增加DDI合增加了短暂PL振荡的数量和宽度.
- *强大的DDI合导致PL峰值的分裂,产生不同的ON/OFF状态.
结论:
- *纳米波导体中的短暂光发光可通过SPP和DDI合控制.
- *观察到的峰值分裂为制造光学纳米开关提供了一个机制.
- *这些发现为开发新型过渡纳米级等离子体设备,如纳米探测器和光学开关铺平了道路.
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