相互作用范围对有吸引力的合体系统的微观结构和动态的作用
Deepak Mangal1, Safa Jamali1,2
1Department of Mechanical and Industrial Engineering, Northeastern University, Boston 02115, USA. s.jamali@northeastern.edu.
Soft matter
|May 24, 2024
概括
粒子吸引的范围显著影响着体系统,从网络转变结构为集群. 这一发现重新定义了长距离相互作用的合凝相界限.
科学领域:
- 体和接口科学科学
- 软物质物理学 软物质物理学
- 材料科学 材料科学 材料科学
背景情况:
- 体凝相图传统上考虑粒子体积分数,吸引力和范围.
- 大多数研究都集中在短距离相互作用上,使得吸引范围的影响不那么被探索.
- 了解体系统动力学和微观结构对于材料设计至关重要.
研究的目的:
- 研究吸引范围对合体系统的微观结构和动态的影响.
- 为了探索不同的吸引范围如何影响弱吸引和强吸引的合体.
- 为具有远程吸引力的合体建立新的凝阶段边界.
主要方法:
- 利用布朗动力学模拟来建模体相互作用.
- 在不同的吸引力范围内分析了合体系统的微观结构和动态.
- 在具有不同吸引力强度和范围的系统中比较凝结速率和最终结构.
主要成果:
- 发现凝结率主要取决于吸引力的强度,而不是范围.
- 吸引范围的增加促使结构性从连接网络向密集集群的过渡.
- 这种过渡发生在弱吸引力和强吸引力体系统中.
结论:
- 吸引范围在确定合凝的最终微观结构方面起着至关重要的作用.
- 对于具有远程吸引力的系统,出现了一个新的合凝阶段边界.
- 模拟结果为设计和预测复杂的体材料的行为提供了洞察力.
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