通过晶格模型模拟,将脆弱到强的过渡与脆弱的玻璃联系起来
Chin-Yuan Ong1, Chun-Shing Lee1,2, Xin-Yuan Gao1
1Department of Applied Physics, Hong Kong Polytechnic University, Hong Kong, China.
Physical review. E
|June 22, 2024
概括
本研究探讨了使用格子模型在玻璃成型器中从脆弱变强 (FTS) 的过渡. 在双模相互作用分布中缩小能量分散会诱导FTS过渡,在温度最小化拉伸指数的温度下观察到.
科学领域:
- 材料科学 材料科学 材料科学
- 凝聚物质物理学 凝聚物质物理学
- 物理化学 物理化学
背景情况:
- 玻璃成型器根据温度依赖的放松率被分为强或脆弱.
- 一些材料,如水,表现出脆弱到强 (FTS) 过渡,在高温和低温下表现不同.
研究的目的:
- 研究玻璃成型器中脆弱到强度 (FTS) 过渡的机制.
- 用可区分粒子格子模型模拟和分析FTS过渡.
主要方法:
- 使用可辨别粒子格子模型,能够模拟强和脆弱的玻璃.
- 启动了与脆弱眼镜特有的双模对相互作用分布的模拟.
- 修改了相互作用分布的低能量组件内的能量分散.
主要成果:
- 通过缩小低能相互作用组件中的能量分散,观察到一个脆弱到强的 (FTS) 过渡.
- 在特定的温度下,FTS过渡发生了,在那里,放松的伸展指数达到最小值.
- 结果与分子动力学模拟的先前发现一致.
结论:
- 能源格局的特点,特别是低能耗组件的分散,对于FTS过渡至关重要.
- 格子模型有效地重现了在实验和模拟研究中观察到的FTS过渡现象.
- 这项工作为管理玻璃过渡行为的基本物理提供了洞察力.
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