在水产养殖湖泊沉积物中的分布特征和释放机制
Xiangyu He1, Wenming Yan1, Xiang Chen2
1The National Key Laboratory of Water Disaster Prevention, Hohai University, Nanjing 210098, China; College of Hydrology and Water Resources, Hohai University, Nanjing 210098, China.
水产养殖通过改变微生物群落和铁/矿物质,显著增加了湖泊沉积物中 (As) 的释放. 这项研究揭示了水产养殖增强了As流,影响了沉积物地质化学.
科学领域:
- 环境化学环境化学
- 水生生态学 水生生态学
- 地质化学 地质化学
背景情况:
- 水产养殖改变了湖泊沉积物和微观环境.
- 水产养殖对 (As) 转换的影响机制尚不清楚.
研究的目的:
- 调查阳湖的沉积物A变化.
- 评估化学转化,释放流和机制.
- 确定水产养殖在释中的作用.
主要方法:
- 分析了沉积物孔水中的空间差异As度.
- 在沉积物-水界面 (SWI) 的量化A释放流.
- 利用部分最小平方路径建模 (PLSPM) 来识别影响因素.
主要成果:
- 观察到溶解As度的显著空间变化.
- 随着释放流量从1.32到112.09μg/L不等,在水产养殖地区最高.
- 有机物受到微生物群落和Fe/Mn矿物质的影响.
结论:
- 水产养殖增强了从沉积物中释放的As.
- 铁氧化物结合的甲转化为吸附的甲增加了甲释放潜力.
- 微生物减少和氧化铁溶解有助于在SWI中溶解A的升高.
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