碳酸盐和有机物质在酸盐占主导地位的热带流域中的意想不到的贡献:同位素方法
Sachintha Senarathne1, Robert van Geldern1, Rohana Chandrajith2
1Friedrich-Alexander-Universität Erlangen-Nürnberg (FAU), Department Geographie und Geowissenschaften, 91054 Erlangen, GeoZentrum Nordbayern, Schlossgarten 5, Germany.
The Science of the total environment
|July 11, 2024
概括
热带河流是碳循环中的重要参与者. 岩石气候变化和有机物循环是关键组成部分,影响这些生态系统中的大气二氧化碳水平.
科学领域:
- 地质化学 地质化学
- 生物地质化学生物地质化学
- 环境科学 环境科学
背景情况:
- 全球碳循环的理解往往忽视了小规模的热带河流盆地.
- 热带河流在区域和全球碳预算中发挥着至关重要的作用.
- 晶体酸盐地形对碳循环研究提出了独特的挑战.
研究的目的:
- 研究岩石气候变化和有机物循环在碳循环中的作用.
- 量化碳相 (溶解的无机碳,溶解的有机碳,有机碳颗粒) 和它们的同位素特征.
- 确定不同来源在酸盐占主导地位的流域中对河流碳池的贡献.
主要方法:
- 溶解和颗粒碳的地球化学分析.
- 碳相的稳定碳同位素分析 (δ13C).
- 同位素质量平衡建模,考虑脱气和光合作用.
主要成果:
- 溶解无机碳 (DIC) 在碳池中占主导地位 (6789%).
- δ13C-DIC值在-11.1至-16.5‰之间,表明来源混合.
- 碳酸盐气候变化和有机物流动对DIC有显著的贡献 (高达60%),即使是在酸盐占主导地位的地区.
结论:
- 岩石气候变化和有机物循环对于热带河流的碳循环至关重要.
- 德杜鲁·奥亚河 (Deduru Oya River) 作为大气二氧化碳的净来源.
- 二氧化碳脱气和光合作用是热带河流碳运输和转移的关键因素.
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