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药品的催化臭氧化使用CeO₂-CeTiO_x-杂交流超透陶膜

Nikoletta Tsiarta^1,2,3, Silvia Morović⁴, Vilko Mandić⁴

¹Catalan Institute of Water Research, Carrer Emili Grahit 101, 17003 Girona, Spain.

Nanomaterials (Basel, Switzerland)

|July 13, 2024

概括

一种新的混合臭氧化膜过工艺有效降解了废水中的持久有机微污染物 (OMP). 用CeO2和CeTiOx合的陶膜显示出有希望的结果,尽管复杂的水矩阵提出了挑战.

科学领域:

环境科学环境科学
材料科学材料科学材料科学
化学工程是化学工程的重要组成部分.

背景情况:

废水废水中的持久性有机微污染物 (OMP) 对水的再利用构成风险.
传统的处理方法难以去除这些反抗性污染物.
先进的氧化工艺与膜过相结合,提供了潜在的解决方案.

研究的目的:

评估混合臭氧化膜过 (HOMF) 过程用于OMP去除.
研究用CeO2和CeTiOx合的陶膜的疗效.
评估废矿水和二次废水中的性能.

主要方法:

用CeO2,CeTiOx或两者添加的陶横流超膜 (300kDa MWCO) 的制造.
通过基于溶液的方法和真空透,对催化纳米颗粒的均沉积.
测试OMP降解使用四种模型化合物 (卡巴马泽平,迪克洛菲纳克,布洛芬,PCBA) 在去矿化水和二次废水中.

主要成果:

金属氧化物的成功透到陶膜上,具有不同的透性.
在非矿物化水中使用CeO2 + CeTiOx合膜观察到的最高OMP降解,表明基形成.
由于矩阵干扰,二次废水中降低了降解效率,突出了吸附效应.

结论:

使用化陶膜的HOMF工艺显示了OMP去除的潜力.
对复杂的水矩阵来说,优化的膜兴奋剂和操作条件至关重要.
需要进一步的研究来应对二次废水组成所带来的挑战.

关键词:

催化臭氧化催化臭氧化陶膜是一种陶膜.交叉流过的过方法混合工艺是一个混合工艺.基基是基基的重要组成部分.

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