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Updated: Jun 21, 2025

Synthesis and Performance Characterizations of Transition Metal Single Atom Catalyst for Electrochemical CO2 Reduction
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Synthesis and Performance Characterizations of Transition Metal Single Atom Catalyst for Electrochemical CO2 Reduction

Published on: April 10, 2018

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通过控制局部H2O/CO2比率,在高速率下进行选择性和稳定的CO2电还原

Junmei Chen1, Haoran Qiu1,2, Yilin Zhao1

  • 1Department of Chemical and Biomolecular Engineering, National University of Singapore, Engineering Drive 4, Singapore, 117585, Singapore.

Nature communications
|July 13, 2024
PubMed
概括

在催化剂接口上精确控制水和二氧化碳度是有效电化学二氧化碳减排的关键. 薄聚合物涂层有效调整这些度,提高多碳产品的产量和稳定性.

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Controlled-potential coulometry, also known as potentiostatic coulometry, employs a three-electrode system in which the working electrode's potential is precisely regulated using a potentiostat. Platinum working electrodes are utilized for positive potentials, while mercury pool electrodes are favored for extremely negative potentials. The platinum counter electrode is separated from the analyte using a membrane or salt bridge to avoid interference in the analysis.
The chosen potential...
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In a galvanic cell, the electrical work is done by a redox system on its surroundings as electrons produced by the spontaneous redox reactions are transferred through an external circuit. Alternatively, an external circuit does work on a redox system by imposing a voltage sufficient to drive an otherwise nonspontaneous reaction in a process known as electrolysis. For instance, recharging a battery involves the use of an external power source to drive the spontaneous (discharge) cell reaction in...
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