黑色碳在Pyrocumulonimbus云中的光吸收增强
Payton Beeler1,2, Joshin Kumar1, Joshua P Schwarz3
1Center for Aerosol Science and Engineering, Department of Energy, Environmental and Chemical Engineering, Washington University in St. Louis, St. Louis, MO, USA.
Nature communications
|July 25, 2024
概括
热 (pyroCb) 火风暴将黑碳 (BC) 注入平流层. 这项研究量化了BC粒子的吸收增强因子,发现它在厚厚的涂层下与2.0不对称.
科学领域:
- 大气化学 大气化学
- 气溶科学 气溶科学
- 气候科学 气候科学
背景情况:
- 热 (pyroCb) 火风暴将大量的黑碳 (BC) 注入平流层,影响大气组成和温度.
- 来自pyroCb事件的BC粒子具有厚厚的有机涂层,可以增强光吸收.
- 对pyroCb BC的吸收增强因子 (Eabs) 没有很好的约束,限制了准确的气候建模.
研究的目的:
- 在pyroCb云中对BC属性的粒子尺度测量.
- 使用已建立的光学模型量化pyroCb BC的吸收增强因子 (Eabs).
- 为在pyroCb事件中提供BC吸收的观察约束参数.
主要方法:
- 在现场测量BC质量,形态和 pyroCb 云中的涂层厚度.
- 应用一个粒子分辨率的BC光学模型来量化Eabs.
- 分析涂层厚度与Eabs.之间的关系.
主要成果:
- 随着涂层厚度的增加,BC的总体平均Eabs对比为2.0.
- 这个值代表了大气中厚层BC的Eabs上限.
- 观察到的BC粒子呈现出厚厚的有机表面涂层.
结论:
- 来自pyroCb事件的厚层BC显著增强光吸收,上限Eabs为2.0.
- 这些发现有助于更好地了解BC从火灾风暴中产生的辐射影响.
- 结果使气候模型中pyroCb事件的辐射转移计算更加精确.
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