在6R-TaS_{2}中,超导的压力诱导非单调演变具有自然批量范德瓦尔斯异构结构
Shaopeng Wang1,2, Yuyan Han1, Sutao Sun3
1Anhui Key Laboratory of Low-energy Quantum Materials and Devices, <a href="https://ror.org/01gh88804">High Magnetic Field Laboratory</a>, HFIPS, Chinese Academy of Sciences, Hefei 230031, China.
Physical review letters
|August 19, 2024
概括
高压抑制电荷密度波 (CDW) 顺序在6R-TaS_{2},影响超导 (SC). 超导性与CDW波动有关,这表明约瑟夫森合效应在这种分层材料中存在.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 固态化学 固态化学
背景情况:
- 6R-TaS_{2}是一种自然的范德瓦尔斯异构结构,具有交替的1T-和1H-TaS_{2}单层.
- 这种独特的结构包含了电荷密度波 (CDW) 顺序和超导 (SC) 在单独的层中.
研究的目的:
- 在高压下研究CDW和SC在6R-TaS_{2}中的演变.
- 了解CDW顺序和超导性之间的相互作用,在这个分层材料.
主要方法:
- 在6R-TaS_{2}上进行了高压电子传输测量.
- 据证实,格子的二维性质可以保存到8GPa.
主要成果:
- 在1T层中的CDW顺序随着压力增加而逐渐被抑制.
- 超导体表现出圆顶形的行为,在约2.9 GPa的临界压力 (P_{c}) 结束.
- SC抑制与CDW崩相关,表明约瑟夫森合效应.
结论:
- 6R-TaS_{2}表现得像堆叠的约瑟夫森结,SC受CDW波动的影响.
- 在CDW在P_{c}以上化后,在1T层中形成新兴超导.
- 6R-TaS_{2} 作为研究竞争电子状态和新兴现象的模型系统.
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