使用机器学习和响应表面方法论分析结构包装柱中的有效面积和质量转移
Amirsoheil Foroughi1, Kamyar Naderi1, Ahad Ghaemi2
1School of Chemical, Petroleum and Gas Engineering, Iran University of Science and Technology, Narmak, Tehran, 16846, Iran.
Scientific reports
|August 24, 2024
概括
机器学习 (ML) 和响应表面方法 (RSM) 用于模拟二氧化碳吸收列中的质量转移系数. ML模型,特别是RBF和MLP,在微分有效面积,气体和液相质量转移系数方面表现出比RSM更好的预测能力.
科学领域:
- 化学工程是化学工程的重要组成部分.
- 质量转移是指质量转移.
- 过程建模过程建模
背景情况:
- 准确预测质量转移系数对于设计高效的二氧化碳吸收列至关重要.
- 结构化包装显著影响质量转移性能.
- 像响应表面方法 (RSM) 这样的传统方法在捕捉复杂关系方面存在局限性.
研究的目的:
- 开发和比较机器学习 (ML) 模型和RSM,用于预测结构化二氧化碳吸收列中的质量转移系数 (微分有效面积,气相和液相).
- 确定影响质量转移的包装的关键结构参数.
- 评估ML模型对RSM的预测优势.
主要方法:
- 利用了四个结构化的包装特征:表面积 (ap),波纹角度 (θ),通道底部 (B) 和高 (h).
- 使用响应表面方法 (RSM) 开发了相关性.
- 采用了五种机器学习模型:随机森林 (RF),辐射基函数神经网络 (RBF),多层感知器 (MLP),XGB回归器和额外树木回归器 (ETR).
主要成果:
- RSM推导了具有高确定系数 (R2) 的相关性:af为0.9717;kG为0.9907;kL为0.9323 .
- ML模型表现出色:af (R2=0.9813) 和kG (R2=0.9933) 的RBF,kl (R2=0.9871) 的MLP.
- 包装道底部 (B) 受影响最大 af 和 kL,而高 (h) 受影响最大 kG.
结论:
- 与RSM相比,机器学习模型,特别是RBF和MLP,对于质量转移系数提供了更高的预测精度.
- 该研究成功地确定了影响结构包装中质量转移的关键结构参数.
- 开发的ML模型为优化二氧化碳吸收柱设计提供了一个强大的工具.
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