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在活跃的布朗硬盘中重新进入的透
David Evans1, José Martín-Roca2,3, Nathan J Harmer1
1Department of Chemistry, Durham University, South Road, Durham DH1 3LE, UK. m.a.miller@durham.ac.uk.
Soft matter
|September 12, 2024
概括
活性物质的聚合和透表现出复杂的行为. 增加的活动最初有助于集群形成,但后来导致分裂,导致相隔之前的非单调透值.
科学领域:
- 物理 物理学 物理
- 统计力学 统计力学
- 软物质物理学 软物质物理学
背景情况:
- 活性物质系统表现出独特的集体行为,与平衡系统不同.
- 机动性诱导的相分离 (MIPS) 是活性物质中的一个关键现象,由自我推进驱动.
- 了解非平衡集群和透对于活性物质动态至关重要.
研究的目的:
- 在2D活性物质模型中研究非平衡聚类和透.
- 分析活动对集群形成和透值的影响.
- 探索从单相向运动性诱导相分离的过渡.
主要方法:
- 自行推进的布朗反射粒子的动态模拟.
- 在MIPS之前对单相区域的分析.
- 应用代的博尔兹曼倒置来导出有效潜力.
- 与被动系统的蒙特卡洛模拟进行比较.
主要成果:
- 较弱的活动增强了集群形成,降低了透值.
- 较高的活动水平导致由于竞争吸引力和集群解体而导致重新进入的透.
- 观察到系统跨度集群的最小临界密度.
- 高阶结构相关性中的差异,而不是辐射分布函数,决定了透灵敏度.
结论:
- 在MIPS前的状态下,活性物质表现出非单调的透行为.
- 活动驱动的力量创造了复杂的结构,这些结构不能完全被平衡模型所捕捉.
- 高阶相关性对于理解活跃系统中的透至关重要.
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