中心对称半导体中的圆形光电流具有隐藏的自旋极化
Kexin Wang1, Butian Zhang2, Chengyu Yan1
1MOE Key Laboratory of Fundamental Physical Quantities Measurement and Hubei Key Laboratory of Gravitation and Quantum Physics, PGMF and School of Physics, Huazhong University of Science and Technology, Wuhan, 430074, China.
Nature communications
|October 19, 2024
概括
隐藏自旋偏振的中心对称材料可以产生自旋偏振的圆形光电流. 这一突破使得通过使用量身定制的光线打破全球反向对称性,使得自旋电子设备的应用成为可能.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 这就是Spintronics.
背景情况:
- 具有位点反向不对称的中心对称材料表现出隐藏的旋转极化,由于保留了全局反向对称性,很难转化为旋转电流.
- 现有的旋转电流生成方法通常需要打破全局逆向对称或应用电偏差.
研究的目的:
- 为了在没有电偏差的中心对称过渡金属二二半导体中演示旋极化的圆形光电流.
- 探索使用空间变化的循环极化光产生自旋梯度和循环电流的机制.
- 为了利用圆形光电流来探测旋转极化和反旋转霍尔效应.
主要方法:
- 利用空间变化的循环极化光来打破中心对称材料中的全球反向对称性.
- 研究圆形光电流对电极配置,照明位置和光束点大小的依赖.
- 在不同的激发波长和温度下使用圆形光流来探测旋转偏振和逆旋转霍尔效应.
主要成果:
- 在正常发生率下,成功地在中心对称过渡金属二二二氧化物半导体中产生了自旋极化圆形光电流.
- 证明空间不均的光会打破全球反转对称性,通过反转霍尔效应诱导旋转梯度和循环电流.
- 建立了一种方法来探测隐藏的旋转偏振和反旋转霍尔效应,使用圆形光电流.
结论:
- 具有隐藏的自旋偏振和不消失的果曲率的中心对称材料对于自旋电子设备应用是可行的.
- 空间变化的循环极化光提供了一种新的途径,可以在中心对称材料中产生和控制自旋电流.
- 展示的光电流生成和探测技术为先进的自旋电子功能开辟了新的途径.
相关概念视频
π Electron Effects on Chemical Shift: Aromatic and Antiaromatic Compounds
1.2K
In aromatic compounds, such as benzene, the circulation of (4n + 2) π-electrons sets up a diamagnetic or diatropic ring current around the perimeter of the molecule. This current induces a magnetic field that opposes the external field inside the ring and reinforces it on the outside. The protons in benzene are deshielded and exhibit high chemical shifts in the range 6.5–8.5 ppm. The shielding effect at the center of the ring is evident in complex aromatic molecules, such as...
1.2K
Atomic Nuclei: Nuclear Spin State Overview
888
NMR-active nuclei have energy levels called 'spin states' that are associated with the orientations of their nuclear magnetic moments. In the absence of a magnetic field, the nuclear magnetic moments are randomly oriented, and the spin states are degenerate. When an external magnetic field is applied, the spin states have only 2 + 1 orientations available to them. A proton with = ½ has two available orientations. Similarly, for a quadrupolar nucleus with a nuclear spin value of...
888
Biasing of P-N Junction
437
The operation of a p-n junction diode involves various biasing conditions, including forward bias, reverse bias, and equilibrium.
In equilibrium, no external voltage is applied across the p-n junction. The depletion region is formed at the junction interface due to the diffusion of carriers, which leaves behind charged dopants, acceptors on the p-side, and donors on the n-side. These immobile charges create an electric field that prevents further diffusion of carriers. The related energy band...
In equilibrium, no external voltage is applied across the p-n junction. The depletion region is formed at the junction interface due to the diffusion of carriers, which leaves behind charged dopants, acceptors on the p-side, and donors on the n-side. These immobile charges create an electric field that prevents further diffusion of carriers. The related energy band...
437
Induced Electric Dipoles
4.2K
A permanent electric dipole orients itself along an external electric field. This rotation can be quantified by defining the potential energy because the external torque does work in rotating it. Then, the potential energy is minimum at the parallel configuration and maximum at the antiparallel configuration. While the former is a stable equilibrium, the latter is an unstable equilibrium.
Since the absolute value of potential energy holds no physical meaning, its zero value can be chosen as per...
Since the absolute value of potential energy holds no physical meaning, its zero value can be chosen as per...
4.2K
Biasing of Metal-Semiconductor Junctions
215
Biasing metal-semiconductor junctions involves applying a voltage across the junction. Specifically, the metal is connected to a voltage source, while the semiconductor is grounded. This technique is essential for controlling the direction and magnitude of current flow in electronic devices, including diodes, transistors, and photovoltaic cells.
In Schottky junctions, where the semiconductor is n-type, applying a positive voltage to the metal relative to the semiconductor reduces its Fermi...
In Schottky junctions, where the semiconductor is n-type, applying a positive voltage to the metal relative to the semiconductor reduces its Fermi...
215
Photochemical Electrocyclic Reactions: Stereochemistry
1.8K
The absorption of UV–visible light by conjugated systems causes the promotion of an electron from the ground state to the excited state. Consequently, photochemical electrocyclic reactions proceed via the excited-state HOMO rather than the ground-state HOMO. Since the ground- and excited-state HOMOs have different symmetries, the stereochemical outcome of electrocyclic reactions depends on the mode of activation; i.e., thermal or photochemical.
Selection Rules: Photochemical Activation
Selection Rules: Photochemical Activation
1.8K


