评估在混合培养工艺中在低C/N条件下在PHA积累阶段内部再利用含废水的效率和潜力
Qingyan Lv1, Hanwen Gao1, Long Huang1
1School of Ecology and Environment, Zhengzhou University, Zhengzhou 450001, China.
Bioresource technology
|January 1, 2025
概括
这项研究表明,在从废弃生物质中生产聚酸酸盐 (PHA) 时,氨的有效再利用. 优化条件显著提高PHA产量,同时减少能源使用和排放.
科学领域:
- 生物技术和生物化学工程 生物技术和生物化学工程
- 环境科学与工程环境科学与工程
- 聚合物科学 聚合物科学
背景情况:
- 聚酸酸 (PHAs) 为传统塑料提供一种可生物降解的替代品.
- 基于混合培养 (MC) 的PHA生产面临来自氨抑制的挑战,影响产量和能源效率.
- 从废物生物质中有效的碳回收对于可持续的PHA合成至关重要.
研究的目的:
- 研究PHA生产中有效的氨二氧化再利用策略.
- 为了减轻氨对PHA产量和能源消耗的抑制作用.
- 为了防止与氨排放相关的二次污染.
主要方法:
- 使用各种混合培养类型,基质组成,养策略和氧气水平进行了PHA生产试验.
- 该研究将条件优化为富含酸盐,高负荷,低氧模式 (R_BC(4) P(1) O(+)).
- 在生产PHA的MC丰富系统中测试了含氨的废水的直接回收.
主要成果:
- 优化模式 (R_BC(4) P(1) O(+)) 实现了0.45g COD/g COD的PHA转换比率,比比较模式高1.8倍.
- 氨吸收达到0.06g NH3-N/g PHA,生产率为4.54g/L,表明有效的回收.
- 直接废水回收没有显著的负面影响到MC流的特性或PHA合成能力.
结论:
- 高效的氨重复利用是可行的,对PHA生产有利.
- 优化的工艺条件提高PHA产量,减少能源消耗,降低二氧化碳排放.
- 在回收废水中溶解的微生物产品对用于PHA合成的MC丰富具有最小的不良影响.
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