在河湖连接系统的沉积物中竞争下的源-沉积动力学
Yongsheng Chang1, Wang Shuhang2, Feifei Che2
1College of Environmental Science and Engineering, Donghua University, Shanghai, 201620, China.
Environmental science. Processes & impacts
|February 17, 2025
概括
河流是连接湖泊的 (As) 污染的重要来源. 河流和湖泊地区的沉积物对释放的风险很高,受竞争和微生物活动的影响.
科学领域:
- 环境化学环境化学
- 地质化学 地质化学
- 微生物学 微生物学
背景情况:
- 连接河湖系统是复杂的环境,在复杂的环境中, (As) 的运输和转化受到多种因素的影响.
- (P) 竞争对沉积物中的的行为产生重大影响,影响其释放和封存.
- 了解河流和湖泊沉积物中As和P的空间动态对于评估环境风险至关重要.
研究的目的:
- 分析 (As) 源和沉积在 (P) 竞争下沉积物的沉积 (As) 源和沉积的特性,在连接的河湖系统内.
- 调查从河流 (R),湖泊 (L) 和湖中心 (LC) 区域的沉积物中释放的酸盐的区域性和连续性.
- 确定控制As释放的因素,包括沉积物特性,P竞争和微生物群落组成.
主要方法:
- 对沉积物质的分析,包括氧化降解潜力 (ORP),pH,以及度的分析.
- 确定As和P的释放潜力 (EAsC0,EPC0) 和As和度 (DAsS).
- 使用16S rRNA测序进行微生物社区分析,以确定主导物种及其与As释放的相关性.
主要成果:
- 沉积物表现出负的ORP,表明减少条件. 河流沉积物是酸性的,而湖中沉积物是性的.
- R区域充当了强大的As源和弱的P源,而LC区域则是As sink和P源. 在R和L地区确定了高As释放风险.
- 在沉积物中丰富的蛋白质细菌与As释放风险呈正相关性. 表面沉积物对释放作出了最重要的贡献,释量超过释量.
结论:
- 河流是连接湖泊的污染的重要贡献者,在不同区域具有不同的As和P动态.
- 沉积物质,P竞争和微生物群落 (特别是蛋白质细菌) 在调节As释放和封存方面发挥着关键作用.
- 管理策略应考虑污染的空间异质性,并在河湖系统内释放风险.
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