通过特拉赫兹发射光谱学揭示石墨烯/MoS2异构结构中的非线性光流
Yifan Cheng1, Xian Lin1, Chunwei Wang2,3
1Department of Physics, Shanghai University, Shanghai 200444, China.
The journal of physical chemistry letters
|March 6, 2025
概括
石墨烯和过渡金属二甲基化物异构结构显示出协同非线性效应. 接口电荷转移和光子阻力效应有助于这些新型光电子材料的太赫兹辐射.
科学领域:
- 光电学是指光电子产品.
- 材料科学 材料科学 材料科学
- 凝聚物质物理学 凝聚物质物理学
背景情况:
- 石墨烯 (Gr) 和过渡金属二甲基化物 (TMDs) 的异构结构对光电子有希望.
- 对界面电荷转移 (CT) 的研究广泛,但对非线性效应的探索较少.
研究的目的:
- 在Gr/MoS2异构结构中研究界面CT和非线性光电流之间的协同相互作用.
- 描述Gr/MoS2和MoS2/Gr/MoS2系统中的太赫兹 (THz) 发射机制.
主要方法:
- 使用的特拉赫兹 (THz) 辐射光谱.
- 进行了各种流动,亚齐木图角,冲击角和极化状态的实验.
主要成果:
- 尽管取消了CT光电流,但在MoS2/Gr/MoS2异构中观察到THz排放,表明了其他贡献.
- 确定光子阻力效应 (PDE) 在MoS2/Gr/MoS2中主导THz发射,特别是光子阻力注入电流.
- 发现CT和PDE都对Gr/MoS2中的THz排放有所贡献,CT占主导地位 (5:2比).
结论:
- 在Gr/MoS2异构结构中证明了界面CT和非线性光电流之间的协同作用.
- 确定了主导的THz发射机制 (MoS2/Gr/MoS2中的PDE,Gr/MoS2中的CT和PDE).
- 建立了开发基于这些异构结构的下一代光电子设备的基础.
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