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释放水性离子电池的潜力:通过双功能调节器辅助电解质工程来构建混合性SEI

Shi Wang^1,2, Junjie Li¹, Binze Yang¹

¹State Key Laboratory of Coordination Chemistry, MOE Key Laboratory of Mesoscopic Chemistry, MOE Key Laboratory of High Performance Polymer Materials and Technology, Jiangsu Key Laboratory of Advanced Organic Materials, Suzhou Key Laboratory of Green Intelligent Manufacturing of New Energy Materials and Devices, Tianchang New Materials and Energy Technology Research Center, Institute of Green Chemistry and Engineering, School of Chemistry and Chemical Engineering, Nanjing University, 163 Xianlin Avenue, Qixia District, Nanjing, Jiangsu 210023, P. R. China.

|March 25, 2025

概括

这项研究引入了一种含有阿斯巴甜的新型水性电解质,通过防止不均的沉积和副作用反应来提高水性离子电池的安全性和性能,从而使长时间的能量储存成为可能.

科学领域:

电化学电化学电化学
材料科学材料科学材料科学
储能储能储能储能储能储能

背景情况:

水性离子电池 (AZIB) 提供安全和经济高效的能源存储.
挑战包括不均的沉积和阳极副作用反应,阻碍了AZIB的实际应用.

研究的目的:

开发一种中度的水性电解质,配有双功能调节器,以提高AZIB的性能.
解决沉积不均和阳极接口副作用问题.

主要方法:

使用了一种中度度的酸电解质与阿斯巴甜.
使用实验验证和理论计算.
研究了混合固体电解质接口 (SEI) 的形成.

主要成果:

含有阿斯巴甜的电解质形成了一个强大的混合SEI与ZnF和ZnS.
实现了密集的沉积,使得无树涂层/脱落和出色的可逆性.
演示了一个ZnRadV2O5全电池,容量为240mAhg-1在5Ag-1的8000个循环中.

结论:

开发的电解质有效调节Zn2+溶解,并优化金属分子接口.
这种方法使得高性能和稳定的AZIB成为可能.
为先进的AZIBs提供了关于解决和接口工程的见解.

关键词:

水性离子电池的水性离子电池生物相容的添加剂添加剂中等度的水性电解质.溶解和界面工程的解决方法

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