实地观测重要的非激活 云对黑碳进行清理
Shuo Ding1, Dantong Liu2, Shitong Zhao2
1Department of Environmental Engineering, College of Energy Environment and Safety Engineering, China Jiliang University, Hangzhou 310018, China.
Environmental science & technology
|May 6, 2025
概括
含有黑碳 (BCc) 的气溶通过碰撞/凝聚被云层清理,而不仅仅是云凝聚核 (CCN) 的激活. 这一过程在较大的云滴中更有效,影响BC去除.
科学领域:
- 大气化学 大气化学
- 气溶科学 气溶科学
- 云物理 云物理
背景情况:
- 在云中的清理对于大气气溶的去除至关重要.
- 含有气溶的黑碳 (BCc) 是重要的空气污染物.
- 云凝聚核 (CCN) 激活是传统上接受的BCc.BCc.的主要湿清理机制.
研究的目的:
- 调查和量化BCc在云层中的清理机制.
- 通过CCN激活进行BCc扫描与其他过程之间的区别.
- 了解云滴大小对BCc湿移除的影响.
主要方法:
- 用颗粒分辨率测量BCc混合状态在orographic云残留物中的测量.
- 使用了地面反流虚拟冲击器.
- 在现场测量和显微镜成像云滴和BCc.
主要成果:
- 很大一部分 (30-90%) 的BCc通过碰撞/凝聚进入云层,绕过传统的CCN激活.
- 非CCN激活的BCc的比例随着云滴体大小的增加 (随着滴体直径从7.6增长到15.8微米,从40%增加到80%).
- 对较大的水滴而言,碰撞/凝结清理更有效,特别是在较低的超和水平下.
结论:
- 碰撞/凝聚是BCc在云中的湿的主要途径,与CCN激活一起.
- 湿去除BCc的效率很大程度上取决于云滴的大小和超和度.
- 这项研究提供了新的BCc清除途径的量化,这对于大气中的BC去除和老化模型至关重要.
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