关于人类对硫和碳生态化学循环显著影响的河流证据:来自西江河流域的案例研究
Ye Wang1, Xuming Li2, Shilei Li1
1MOE Key Laboratory of Surficial Geochemistry, School of Earth Sciences and Engineering, and Frontier Science Center for Critical Earth Material Cycle, Nanjing University, Nanjing 210023, China.
Journal of hazardous materials
|May 9, 2025
概括
人类产生的硫排放使西江河中的河硫酸盐度在过去30年中增加了三倍,原因是酸雨和矿氧化. 这影响了碳循环,抵消了自然的封存.
科学领域:
- 环境化学环境化学
- 生物地质化学生物地质化学
- 水文学的水文学
背景情况:
- 人类产生的硫排放对硫和碳的生物地球化学循环产生重大影响.
- 关于河流硫酸盐流及其来源的十年级数据有限.
- 捕获规模的化学过程受到人类硫输入的影响.
研究的目的:
- 分析河流硫酸盐流量和西江河源的十年级变化.
- 调查人为硫排放对河流化学的影响.
- 评估对碳生物地球化学循环的影响.
主要方法:
- 为西江河汇编了30年的河流化学数据集 (1985-2015年).
- 采用蒙特卡洛逆转模型来确定溶解的负载源.
- 分析了硫酸盐度和产量的趋势.
主要成果:
- 从1985年到2015年,河流硫酸盐度增加了三倍以上.
- 在30年的时间里,硫酸盐产量增加了两倍以上.
- 酸雨和矿氧化增加的贡献被确定为主要驱动因素.
- 硫酸 - 碳酸盐反应中的加速CO2产量抵消了酸盐气候结.
结论:
- 人类活动对硫和碳的生物地球化学循环有着迅速而显著的影响.
- 西江河由于人为排放导致硫酸盐流量发生实质性变化.
- 该研究强调了环境变化下的硫和碳循环之间的复杂相互作用.
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