在金属玻璃原体中,通过温度扫描X射线光子相关谱学观察到类似液体的与压力驱动的动力学
Maximilian Frey1, Nico Neuber2, Sascha Sebastian Riegler2
1Chair of Metallic Materials, Saarland University, Saarbrücken, Germany. maximilian.frey@uni-saarland.de.
Nature communications
|May 13, 2025
概括
这项研究表明,金属玻璃中的结构性α放松是液态和原子运动的叠加. 这一发现为玻璃过渡动态和材料行为提供了新的见解.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学 材料科学 材料科学
- 物理化学 物理化学
背景情况:
- 超冷液体和玻璃化动态是关键的研究领域.
- 了解原子级运动对于材料科学至关重要.
研究的目的:
- 在不同状态下探测基于Pt的金属玻璃前者的动态.
- 扩大X射线光子相关谱学 (XPCS) 的动态范围.
主要方法:
- 使用温度扫描X射线光子相关谱学 (XPCS).
- 采用先进的探测器技术和第四代同步辐射.
- 覆盖了跨越六个数量级的时间尺度.
主要成果:
- 在玻璃状状态下观察到结构alpha放松,被更快的原子尺度的装饰关系掩盖.
- 将发现解释为异构的液体式和弹道式原子运动的叠加.
- 扩大了XPCS探测的动态范围.
结论:
- 这项研究为玻璃过渡过程中的α放松提供了新的观点.
- 提供了对金属玻璃和软材料异常时衰变的见解.
- 突出了温度扫描XPCS用于研究复杂动态的实用性.
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