在用MnX-GAC (X=Fe或Zn) 增强的建筑湿地中选择性去除:性能,机制和去除途径
Deliang Chen1, Xianwen Fang2, Lu Zhao2
1School of Environment and Geography, Qingdao University, Qingdao, 266071, China.
Journal of environmental management
|May 21, 2025
概括
颗粒状活性碳复合材料 (MnX-GAC) 增强了废水处理的建筑湿地. 这提高了去除的效率,并选择性地增加了气的产量,同时减少了温室气体排放.
科学领域:
- 环境工程 环境工程
- 水处理技术 水处理技术
- 生物地质化学循环的过程
背景情况:
- 建筑湿地 (CWs) 在废水处理方面是有效的,但由于低的脱效率和温室气体排放而扎.
- 提高CW中基质和微生物之间的协同作用是克服这些局限性的关键.
- 颗粒活性炭 (GAC) 是一种常见的CW基板,但其性能可以提高.
研究的目的:
- 开发和评估新型复合材料填充剂 (MnX-GAC) 以提高去除和减少CW中的温室气体排放.
- 研究MnX-GAC对微生物群落和CW中的转化途径的影响.
- 评估MnX-GAC在促进选择性去除和N2选择性的效率.
主要方法:
- 制备颗粒状活性碳支持的Mn基复合材料填充剂 (MnX-GAC,X=Fe或Zn).
- 将MnX-GAC纳入建筑湿地的上下部分.
- 对去除效率,N2O排放,微生物群落结构 (宏基因组分析) 和功能基因丰度的分析.
主要成果:
- MnX-GAC填充剂显著提高了总去除效率,达到77.1%.
- 使用MnX-GAC建造的湿地减少了氧化 (N2O) 排放,并增加了43.4%的 (N2) 选择性.
- MnX-GAC增强了微生物物种间电子转移,刺激了脱微生物 (Anaerolinea,Thauera),并增加了关键转化基因的丰富性.
结论:
- MnX-GAC复合填充剂是一种有前途的策略,可以提高建筑湿地的选择性除性能.
- 增强的性能归因于改善的微生物活动,电子转移和优化的转化通路.
- 这种方法为高效的废水处理和缓解CWs温室气体排放提供了一个新的解决方案.
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