用扭曲光对铁电拓极结构进行操纵.
Nimish P Nazirkar1, Viet Tran2,3, Pascal Bassène2,3
1Department of Materials Science and Engineering, Rensselaer Polytechnic Institute (RPI), Troy, NY, 12180, USA.
Advanced materials (Deerfield Beach, Fla.)
|June 6, 2025
概括
扭曲的紫外线与轨道角动量 (OAM) 控制CsBiNb2O7晶体中的铁电极化. 这种结构光使铁态和拓刺激的确定性操纵成为可能,为可重新配置的设备铺平了道路.
科学领域:
- 凝聚物质物理学 凝聚物质物理学
- 材料科学是一种材料科学.
- 光子学 是一个光子学.
背景情况:
- 控制不平衡状态是一个关键的挑战.
- 特拉赫兹场和软音声模式影响铁电.
- 带有轨道角动量 (OAM) 的扭曲光提供了一条操纵铁电秩序和拓激发的新途径.
研究的目的:
- 使用非共振扭曲紫外线 (UV) 光来证明铁电偏振的控制.
- 研究OAM在操纵铁态和稳定拓刺激中的作用.
- 建立结构光作为铁态状态的决定性控制的工具.
主要方法:
- 使用的准2D CsBiNb2O7 (CBNO) 单晶.
- 使用的非共振扭曲紫外线 (375 nm,800 THz).
- 结合在现场的X射线布拉格连贯衍射成像 (BCDI),扭曲光学拉曼光谱和密度函数理论 (DFT).
主要成果:
- 解决了3D离子位移,应变场和极化变化.
- 观察到光诱导的应变歇斯底里,表明由OAM驱动的非线性,历史依赖的铁弹性切换.
- 记录了离散的,不可逆转的域过渡和稳定非微不足道的域纹理 (-反对,美龙),在OAM删除后仍然存在,显示了记忆效应.
结论:
- 结构光提供了铁态的决定性和可逆控制.
- 展示了OAM驱动的铁弹性切换和拓缺陷稳定.
- 这些发现使得可光学重新配置的非挥发性设备成为可能.
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