在合体凝中屈服:从局部结构到中尺度链断裂和宏观失效
Himangsu Bhaumik1, Tanniemola B Liverpool2, C Patrick Royall3,4,5
1University of Cambridge, Yusuf Hamied Department of Chemistry, Lensfield Road, Cambridge CB2 1EW, United Kingdom.
Physical review. E
|June 19, 2025
概括
数字模拟揭示了颗粒物枯竭凝如何在压力下流动和屈服. 线条断裂事件是可以预测的,将微尺度属性与宏尺度软流连接起来,并证明粘度分叉.
科学领域:
- 软物质物理学 软物质物理学
- 类风病学 类风病学 类风病学
- 材料科学 材料科学 材料科学
背景情况:
- 颗粒物枯竭凝表现出复杂的流动和产生行为.
- 了解这些行为对于预测压力下的材料性能至关重要.
研究的目的:
- 为了数值模拟爬行流和在颗粒物枯竭凝中的产量.
- 描述跨不同长度和时间尺度的断链事件.
- 为了研究微尺度链属性与宏观尺度流动行为之间的关系.
主要方法:
- 在恒定切割应力下,爬行流量的数值模拟.
- 对中大尺度链断裂事件的分析.
- 微观结构和机械指标的时空空间分析.
主要成果:
- 链断裂事件均分布,与软流相对应.
- 微尺度分析表明,链断裂在统计上是可预测的.
- 爬行和衰老动态之间的相互作用导致粘度分叉.
结论:
- 微尺度的链状动力学决定了缩水凝的宏观产量和流量.
- 这项研究为基于基本性质的凝行为预测提供了一个框架.
- 证明了粘度分支,突出了不同的流动模式.
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