DeepNSI:用于非法物质检测的实验光中子光谱中的元素识别
C Besnard-Vauterin1, V Blideanu1, B Rapp2
1Université Paris-Saclay, CEA, List, Laboratoire National Henri Becquerel (LNE-LNHB), F-91120, Palaiseau, France.
概括
深度学习框架DeepNSI使用光子诱导的中子光谱准确识别元素组成,用于检测非法材料. 它提供可靠的元素分析与不确定性估计,以提高决策信心.
科学领域:
- 核物理与工程 核物理与工程
- 材料科学 材料科学 材料科学
- 人工智能的人工智能
背景情况:
- 光子探测系统对于安全应用至关重要,但准确的元素分析仍然具有挑战性.
- 检测和氧等轻元素对于识别爆炸物和化学威胁至关重要.
- 现有的方法往往缺乏复杂的检查场景所需的精度和解释性.
研究的目的:
- 开发一个强大的深度学习框架,DeepNSI,用于从光子诱导的中子光谱中识别元素组成.
- 增强对光元素的检测能力,对于安全应用至关重要.
- 为可靠的决策提供可解释的结果与不确定性量化.
主要方法:
- 开发了DeepNSI,这是一组特定元素的卷积神经网络.
- 在模拟和实验光中子光谱的混合数据集上训练模型.
- 纳入预测不确定性的蒙特卡罗脱落和用于光谱重建的非负最小平方 (NNLS).
主要成果:
- 在现实数据上展示了强大的元素识别,包括有机化合物和屏蔽材料.
- 实现了轻元素的可靠检测,爆炸物和化学威胁的关键签名.
- NNLS趋势反映了有意义的组成差异,支持可解释的分析.
结论:
- DeepNSI提供了一种可靠的,基于机器学习的方法,用于光子查询系统中的元素分析.
- 该框架提供可解释的结果与不确定性估计,增强对安全应用程序的信心.
- DeepNSI在光子中子谱学领域取得了进展,用于材料检查和威胁检测.
相关概念视频
Atomic Emission Spectroscopy: Lab
251
AES is a powerful analytical technique, especially effective when used with plasma sources, producing abundant spectra in characteristic emission lines. The Inductively Coupled Plasma (ICP), in particular, yields superior quantitative analytical data due to its high stability, low noise, low background, and minimal interferences under optimal experimental conditions. However, newer air-operated microwave sources are emerging as promising alternatives that could be more cost-effective than...
251
Mass Spectrum: Interpretation
1.6K
An unknown compound can be established by identifying the molecular ion peak in the mass spectrum. The molecular ion peak is often weak or absent due to the predominance of fragmentation in high-energy electron beams. In such cases, a low-energy electron beam can be used to scan the spectrum to enhance the intensity of the molecular ion peak. Additionally, chemical ionization, field ionization, and desorption ionization spectra are used to obtain a relatively intense molecular ion peak.
To...
To...
1.6K
Atomic Spectroscopy: Absorption, Emission, and Fluorescence
1.3K
Atomic spectroscopy is a vital tool in elemental analysis, both qualitatively and quantitatively. It can be broadly divided into optical spectroscopy, mass spectroscopy, and X-ray spectroscopy methods. The optical spectroscopic methods are atomic absorption spectroscopy (AAS), atomic emission spectroscopy (AES), and atomic fluorescence spectroscopy (AFS). The first step in all three methods is atomization, where the solid, liquid, or solution-phase samples are converted into gas-phase atoms and...
1.3K
Atomic Emission Spectroscopy: Overview
2.6K
Atomic emission spectroscopy (AES) is an analytical technique used to determine the elemental composition of a sample by analyzing the light emitted from excited atoms. In AES, atoms in a sample are excited to higher energy levels by thermal energy from high-temperature sources, such as plasma, arcs, or sparks. When these excited atoms return to lower energy states, they emit light at specific wavelengths characteristic of each element. The resulting atomic emission spectrum, which consists of...
2.6K
Mass Spectrometry: Isotope Effect
2.5K
Most elements exist in nature as a mixture of isotopes. The isotopes differ in weight due to their respective number of neutrons. The molecular weight of a molecule is different depending on the specific isotope of its elements involved. As a result, the mass spectrum of the molecule exhibits peaks from the same fragment at multiple positions. The positions of these mass signals depend on the difference between the molecular mass. Furthermore, the intensity of these signals is dependent on the...
2.5K
Atomic Emission Spectroscopy: Instrumentation
615
The instrumentation of atomic emission spectrometry (AES) involves various components, including atomization devices that convert samples into gas-phase atoms and ions. There are two main types of atomization devices: continuous and discrete atomizers. Continuous atomizers, like plasmas and flames, introduce samples in a constant stream, while discrete atomizers inject individual samples using syringes or autosamplers. The most common discrete atomizer is the electrothermal atomizer.
615


