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生态工程生物聚合物粘土复合物用于酸离子去除:从统计和人工智能建模的协同见解

Rachid Aziam^1,2, Daniela Simina Stefan¹, Safa Nouaa²

¹Department of Analytical Chemistry and Environmental Engineering, Faculty of Chemical Engineering and Biotechnologies, National University of Science and Technology Politehnica of Bucharest, 1-7 Polizu Street, 011061 Bucharest, Romania.

|July 12, 2025

概括

这项研究开发了一种新型的水凝生物复合物,由天然粘土,基酸盐和约塔-卡拉基用于高效的酸盐离子去除. 该材料表现出高吸附能力,并使用响应表面方法和人工神经网络进行了优化.

科学领域:

环境化学环境化学
材料科学材料科学材料科学
水处理处理水的方法

背景情况:

水溶液中的酸盐污染给环境带来了重大挑战.
有效地去除酸离子对于防止肥胖和保持水质至关重要.
开发新型吸附剂是必要的,以实现高效和可持续的酸盐整治.

研究的目的:

通过使用天然粘土,藻酸盐 (Na-AL) 和iota-carrageenan合成一种新的水凝生物复合材料.
为了研究从水溶液中去除酸盐离子的生物复合材料的吸附性能.
使用响应表面方法 (RSM) 优化吸附条件,并使用人工神经网络 (ANN) 预测效率.

主要方法:

使用FTIR,SEM-EDX和零电荷点 (PZC) 进行生物复合材料的表征.
研究吸附动力学,异热和热力学参数.
使用Box-Behnken设计 (BBD-RSM) 优化吸附剂剂量,接触时间和初始度.
人工神经网络 (ANN) 的应用用于预测吸附效率.

主要成果:

这种生物复合材料具有很高的吸附能力:H2PO4-的吸附能力为140.84 mg/g,HPO42-的吸附能力为105.26 mg/g.
伪二次 (PSO) 运动模型最好地描述了吸附过程.
兰穆尔和弗罗恩德利希的异热模型显示出高显著性 (R2 ≈ 1),表明不同的吸附点.
RSM和ANN模型显示出高可靠性和预测能力 (R2 = 0.9714和R2 = 0.974,分别).

结论:

合成的水凝生物复合材料是酸离子的高效吸附剂.
吸附是自发的,内热的,并且涉及固体-液体界面的疾病增加.
使用BBD-RSM进行优化和使用ANN进行预测,为高效的酸盐去除提供了可靠的框架.
这种新材料为减轻水体中酸盐污染提供了有希望的解决方案.

关键词:

一个年龄,一个年龄.在 RSM RSM 中.酸是一种酸.生物复合材料珠子生物复合材料珠子约塔 - - 卡拉基安南.自然的粘土是天然的.酸盐离子酸盐离子

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