在城市环境中的轮胎衍生周期性氨基物质上海的颗粒物质
Munila Abudumutailifu1, Chengze Li1, Haiping Xiong1
1Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention (LAP3), National Observations and Research Station for Wetland Ecosystems of the Yangtze Estuary, Department of Environmental Science & Engineering, Fudan University, Shanghai 200438, China.
概括
轮胎磨损化合物 (TWC) 在城市PM2.5中普遍存在,秋季发现的度最高. 夜间接触这些化合物是显著的,需要进一步的健康影响研究.
科学领域:
- 环境化学环境化学
- 大气科学 大气科学
- 公共卫生 公共卫生
背景情况:
- 轮胎磨损化合物 (TWC) 和它们的副产品是重要的环境污染物.
- 人们对广泛生产和使用轮胎释放的TWC对环境和健康的影响存在担忧.
研究的目的:
- 在城市PM2.5.5中选和量化可疑的TWC.
- 调查TWC的季节性和日间变化.
- 为了检查大气中6PPD-Q与其母化合物6PPD的比例.
主要方法:
- 使用定制的气溶度丰富系统与HPLC-Q-TOF-MS相结合.
- 对十个选定的TWC进行了非有针对性的选和有针对性的量化.
- 收集了夏季,秋季和冬季在上海的高时间分辨率数据.
主要成果:
- 总TWC度 (TWCs) 在秋季 (15.53 ng/m3) 最高,其次是夏季 (7.44 ng/m3) 和冬季 (5.74 ng/m3).
- TWC的季节性贡献在秋季为73.9%,夏季为18.6%,冬季为7.5%.
- 观察到TWC的夜间度升高,6PPD-Q/6PPD比率在下午达到顶峰.
结论:
- 在TWC中,城市PM2.5.5的季节性和日间变化显著.
- 夜间暴露于TWC是公共健康的关键考虑因素.
- 对TWC进行进一步的毒理和流行病学研究是必不可少的.
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