页岩对超临界CO2的反应性:从Caney页岩中微观结构特征和矿物阶段演变的洞察力,用于CCUS应用
Loic Bethel Dje1, Mileva Radonjic1
1Barrier Materials and Geomimicry Lab, School of Chemical Engineering, Oklahoma State University, Stillwater, OK 74078, USA.
超临界二氧化碳 (scCO2) 暴露改变了页岩矿物学,导致碳酸盐溶解和元素再分配. 储页岩显示出多孔性增加,同时保持顶岩完整性,这对于二氧化碳封存安全至关重要.
科学领域:
- 地质化学 地质化学
- 矿物学是一门学科.
- 地质工程是地质工程.
背景情况:
- 了解矿物流体相互作用对于评估二氧化碳 (CO2) 沉积在页岩层中的长期地质化学含量至关重要.
- 页岩构造是复杂的地质系统,具有不同的矿物成分,影响其反应性.
研究的目的:
- 描述Caney页岩样本中的矿物质变化和元素再分配,这些样本暴露于超临界二氧化碳 (scCO2).
- 为了评估scCO2对二氧化碳封存应用的水库和上层岩层的影响.
主要方法:
- 五个卡尼页岩样本 (水库和岩层) 静态暴露于60°C和17.23MPa的纯sCO230天.
- 扫描电子显微镜与能量分散光谱 (SEM-EDS) 分析暴露前后,以确定矿物学和元素变化.
主要成果:
- 暴露后观察到显著的碳酸盐损失 (15-40%在水库中,高达20%在石头岩中).
- 在Illite和K-feldspar中Fe2+,Mg2+和K+的耗尽;与Fe再分配的pyrite氧化;表面变化和对有机物质的吸附效应.
- Ca2+,Mg2+,Fe2+和Si4+的调动;水库样本中局部孔隙的发展;岩样本中结构完整性的保存.
结论:
- scCO2暴露会诱导页岩的矿物学和元素变化,对水库和石头岩层产生不同的影响.
- 观察到的变化为矿物反应性和元素流量提供了关键的见解,这与页岩层中二氧化碳封存的安全性和有效性有关.
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