在有吸引力的合体的凝结和粗化过程中,颗粒网络的出现和演变
Paniz Haghighi1, Mohammad Nabizadeh1, Safa Jamali1,2
1Department of Mechanical and Industrial Engineering, Northeastern University, Boston, MA 02115, USA. s.jamali@northeastern.edu.
Soft matter
|September 15, 2025
概括
凝结在有吸引力的合体中形成一个网络,然后粗化. 这项研究确定了凝作为一个阶段过渡,使用网络演变的定量测量和透和粗的独特结构划界.
科学领域:
- 合体和表面科学科学
- 软物质物理学 软物质物理学
- 材料科学 材料科学 材料科学
背景情况:
- 在有吸引力的合体中凝结涉及网络形成,透和随后的粗.
- 了解这些转变对于控制材料性质至关重要.
研究的目的:
- 引入定量措施,以确定合凝中的关键过渡点.
- 分析凝过程中颗粒网络的形成和演变.
- 区分透和粗化作为不同的过渡.
主要方法:
- 分析状集群动态和网络演变.
- 量化测量 koloid 集群变化速率的量化测量.
- 随着时间的推移,跟踪粒子网络的直径.
- 使用全球结构性措施,如沃罗诺伊体积分布.
主要成果:
- 凝结被确定为通过集群动态的连续第二阶段过渡.
- 网络直径在透过渡时呈现出明显的最大值.
- 当地结构性措施 (例如,协调号) 不反映透.
- 累积粒子接触和沃罗诺伊体积分布标志着粗.
结论:
- 颗粒凝中的透和粗是具有明确结构划分的明显过渡.
- 量化全球测量有效地识别了这些跨越不同条件的转变.
- 这为理解和控制体凝形成提供了一个框架.
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