δ-MnO2-改性花生生物炭和酸促进了Mn(IV) 减少驱动的氧化与Cr(VI) 移除
Yue Wang1, Yihan Bai1, Junfeng Su1
1School of Environmental and Municipal Engineering, Xi'an University of Architecture and Technology, Xi'an 710055, China; Shaanxi Key Laboratory of Environmental Engineering, Xi'an University of Architecture and Technology, Xi'an 710055, China.
Bioresource technology
|September 18, 2025
概括
这项研究使用新型生物炭和酸加强了和的去除,实现了超过97%的和98%的减少. 该方法增强了微生物活动,以有效处理废水.
科学领域:
- 环境微生物学 环境微生物学
- 环境化学环境化学
- 生物技术是生物技术.
背景情况:
- (NH4+-N) 和 (Cr) 是影响水生生态系统的重要废水污染物.
- 涉及NH4+-N氧化与降解相结合的Mnammox工艺提供了一个潜在的治疗策略.
- 提高Mnammox的效率对于有效的污染物清除至关重要.
研究的目的:
- 为了研究Aromatoleum evansii MAY27在通过Mnammox.VI去除NH4+-N和Cr(VI) 的有效性.
- 开发和优化一种新的Mn(IV) 修饰的花生生物炭 (PSB@δ-MnO2),与酸 (HA) 结合,以提高Mnammox的性能.
- 阐明开发系统中污染物去除和微生物反应的基本机制.
主要方法:
- 对Mnammox的pH,C/N比和HA和PSB@δ-MnO2度的动力优化.
- 培育芳香 evansii MAY27和应用HA-PSB@δ-MnO2系统用于废水处理.
- 对污染物去除效率,微生物活动,电子转移,表面价值状态和基因表达的分析.
主要成果:
- 在优化条件下 (pH 6.5,C/N 0.5,40 mg L-1 HA,1100 mg L-1 PSB@δ-MnO2) 产生了97.03%的NH4+-N去除和18.93 mg的L-1 Mn(II) 生产.
- 该HA-PSB@δ-MnO2系统显著增强了微生物活动,能源生产和电子转移.
- 在初始低度 (<1毫克L-1) 的CrVI时,CrVI的效率超过98%和NH4+-N的效率超过93%.
- 通过沉分析和III/II和III的形成,证据证实了 (IV) 和 (VI) 的减少.
- 转录分析显示了微生物代谢的增强和Mn(IV) 减少基因的上调.
结论:
- 该HA-PSB@δ-MnO2系统有效地增强了Mnammox by Aromatoleum evansii MAY27用于同时去除NH4+-N和CrVI.
- 该研究提供了对改善微生物性能和减少污染物的机制性见解.
- 这种方法为处理NH4+-N和Cr(VI) 污染的废水提供了可持续的理论基础.
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