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光催化CO2的金属有机框架减少:进展和前景

Junchuang Feng¹, Shuangshuang Chen¹, Zhiyong Lu¹

¹College of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 210009, China.

ACS applied materials & interfaces

|October 27, 2025

概括

金属有机框架 (MOF) 是人工光合作用的先进材料,有效地将二氧化碳转化为有价值的燃料. 本综述详细介绍了MOF加强二氧化碳减排的战略,推动负碳能源解决方案.

科学领域:

材料科学材料科学材料科学
催化剂是一种催化剂.
可再生能源可再生能源是可再生能源.

背景情况:

化石燃料的依赖推动了全球能源和环境危机.
人工光合作用系统 (APS) 提供负碳解决方案.
金属有机框架 (MOFs) 在光催化二氧化碳减排 (CO2RR) 方面表现有前途.

研究的目的:

审查提高MOF在CO2RR中的光催化性能的策略.
专注于光子采集,电荷转移和多碳产品的产生.
分析MOF中C-C合的结构设计原则.

主要方法:

工程MOF金属节点,有机链接器和孔隙微环境.
评价光吸收,电荷分离和活性站点设计方面的进展.
建立MOF催化剂的结构-属性关系.

主要成果:

MOF提供可调整的架构,以获得卓越的CO2RR选择性,效率和稳定性.
连接器功能化改善了光吸收;导电通道增强了电荷分离.
量身定制的活性位点和孔隙封闭优化动力控制和C-C合.

结论:

MOFs将原子尺度的可调性与二氧化碳转换的宏观催化效率相结合.
本综述为开发高性能MOF光催化剂提供了路线图.
MOF加速向可扩展,太阳能驱动,负碳能源系统的过渡.

关键词:

电子 - 孔分离的分离采集光的修改方法金属-有机的框架.多碳产品是多碳产品.光催化二氧化碳减排的方法

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