解码埋藏的接口:一个协同框架来掌握固态电池的核心挑战.
Weiheng Chen1,2, Jialong Wu3, Ling Li2
1National and Local Joint Engineering Research Center of Reliability Analysis and Testing for Mechanical and Electrical Products, Zhejiang Sci-Tech University, Hangzhou, Zhejiang, 310018, P. R. China.
Small (Weinheim an der Bergstrasse, Germany)
|November 3, 2025
概括
开发全固态电池需要克服固态界面的不稳定性. 结合计算模拟和实验性表征的协同方法是提高储能安全性和性能的关键.
科学领域:
- 材料科学 材料科学 材料科学
- 电化学 电化学 电化学
- 计算化学计算化学
背景情况:
- 全固态电池承诺比离子电池更高的能量密度和安全性.
- 固体-固体接口的不稳定性对它们的发展构成了重大挑战.
- 目前的研究方法不足以解决复杂的界面退化问题.
研究的目的:
- 强调必要的协同方法,整合计算模拟和实验表征.
- 为解决接口问题提出一个层次框架.
- 展示这种综合方法在理解和设计电池接口方面的重要作用.
主要方法:
- 综合计算和实验方法的综述.
- 提出一个四层次的层次结构框架:基础,动态,多规模和智能.
- 详细的案例研究说明了协同方法的应用.
主要成果:
- 协同作用的方法对于阐明离子运输和预测界面反应至关重要.
- 它可以解构 - 二增长的多物理和化学机械故障.
- 该框架通过AI/ML促进了通过AI/ML加速发现和数据分析.
结论:
- 计算和实验方法的协同范式对于全固态电池的开发至关重要.
- 这种综合方法超越了描述性分析,转向了界面的预测性,理性工程.
- 它对于实现下一代储能稳定,高性能接口至关重要.
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