罢工命令的比较形态签名 核取证的氧化物
Nathan J Meigs1, Logan Gibb1, Nick Kurtyka1
1Department of Nuclear Engineering, University of Utah, 110 Central Campus Dr., Suite 2000, Salt Lake City, Utah 84112, United States.
ACS omega
|November 3, 2025
概括
核取证学依赖于对矿石缩物 (UOC) 的表征. 这项研究发现,降水冲击顺序对大多数合成路径的UOC形态有显著的影响,除了二酸 (MDU),为法医归因提供了潜在的可能性.
科学领域:
- 核化学 核化学 核化学
- 材料科学 材料科学 材料科学
- 机器学习应用 机器学习应用
背景情况:
- 核取证对于检测非法放射性材料至关重要.
- 鉴定矿石缩物 (UOC) 对于核安全至关重要.
- 了解UOC合成途径及其产生的特性至关重要.
研究的目的:
- 调查降水冲击顺序如何影响UOC形态.
- 使用机器学习区分合成路线和罢工命令.
- 为了建立形态指纹的法医归因的UOCs.
主要方法:
- 通过四种路径合成的UOCs (U3O8):AUC,ADU,UO4和MDU.
- 使用基于ResNet34的CNN分析SEM图像以提取形态特征.
- 使用机器学习分类来区分合成路线和罢工命令.
主要成果:
- 大多数合成路线都显示出基于罢工顺序 (p < 0.05) 的显著形态差异.
- 在CNN的分析中,AUC,ADU和UO4路线的分辨准确度很高.
- 在MDU路线显示最小的形态变化和缺乏统计学意义 (42-72%的准确性).
结论:
- 罢工顺序对UOC形态的影响是合成路线依赖的.
- 对于AUC,ADU和UO4确定了不同的形态特征,但不是MDU.
- 罢工命令依赖的形态指纹对核法医归因和过程监控有影响.
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