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The high insolubility of some precipitates can result in an unfavorable relative supersaturation. This can lead to colloidal particles with a large surface-to-mass ratio, where adsorption is promoted. For instance, in the precipitation of silver chloride, silver ions are adsorbed on the surface of the colloidal particles, forming a primary layer. This layer attracts ions of opposite charge (such as nitrate ions), forming a diffuse secondary layer of adsorbed ions. This electric double layer...
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Microbiologically Influenced Corrosion (MIC) is a significant form of material degradation caused by the metabolic activities of microorganisms. This phenomenon poses substantial challenges across various industries, including oil and gas, maritime, and water treatment sectors.MIC occurs when microorganisms, such as bacteria, archaea, and fungi, colonize metal surfaces, forming biofilms that alter the local electrochemical environment. These biofilms can lead to the production of corrosive...
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In Situ Neutron Powder Diffraction Using Custom-made Lithium-ion Batteries
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具有高树脂抑制能力的潜在驱动选择性纳米金属沉积启用介面

Hongli Wan1,2, Chi Chen3, Ni Zhang1,2

  • 1Ningbo Institute of Materials Technology & Engineering, Chinese Academy of Sciences, 315201 Ningbo, China.

Journal of the American Chemical Society
|November 21, 2025
PubMed
概括

这项研究引入了一种全固态金属电池 (ASSLB) 的新型介层和阳极策略. 这种方法同时解决空隙形成和树生长问题,提高了低压下电池的稳定性.

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科学领域:

  • 材料科学
  • 电化学
  • 能量储存

背景情况:

  • 全固态金属电池 (ASSLB) 面临的挑战是剥离过程中的空隙形成以及涂层过程中的树生长.
  • 这些问题限制了ASSLB的稳定性,特别是在低堆压下,阻碍了实际应用.

研究的目的:

  • 在ASSLB中同时解决空洞形成和树突生长问题.
  • 在低堆压下开发ASSLB的稳定循环性能.

主要方法:

  • 使用硬碳-Sn (HC-Sn) 介层和LiNa作为阳极.
  • 研究了现场结构转化为Li6PS5Cl/[HC-LixSn]Na/Na/LiNa.
  • 评估了对称细胞性能和完整细胞循环稳定性.

主要成果:

  • 通过HC-Sn中间层和LiNa阳极实现均的沉积和抑制空隙形成.
  • 在低堆压 (2.0 MPa) 下在对称单元中经过1184小时的稳定化/剥离.
  • 一个完整的细胞在1000个循环后表现出90. 0%的容量保留和高可逆容量.

结论:

  • HC-Sn介层和LiNa阳极策略有效地抑制了Li树突和空隙形成.
  • 这种方法使ASSLB在低堆压下保持稳定的循环性能,为实际应用铺平了道路.